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Journal Articles

Journal Articles

Rapid multi-nuclide identification method by simultaneous $$beta$$, $$gamma$$, and X-ray spectrum analysis

Oshima, Masumi*; Goto, Jun*; Hayakawa, Takehito*; Asai, Masato; Kin, Tadahiro*; Shinohara, Hirofumi*

Isotope News, (790), p.19 - 23, 2023/12

When analyzing samples that contain many radionuclides at various concentrations, such as radioactive waste or fuel debris, it is difficult to apply general spectrum analysis methods and is necessary to chemically separate each nuclide before quantifying it. The chemical separation is especially essential for analysis using a liquid scintillation counter (LSC). In this report, the authors explain the newly developed spectral determination method (SDM) in which the entire spectrum is fitted to quantify radioactivity of nuclides mixed in a sample. By applying the SDM to $$beta$$- and X-ray spectrum measured by LSC and $$gamma$$-ray spectrum measured by Ge detector simultaneously, the authors demonstrated that radioactivity of 40 radionuclides mixed in a sample at concentrations varying by two orders could be quantified, which is useful to simplify chemical separation process in radionuclide quantification.

JAEA Reports

Measurement methods for the radioactive source distribution inside reactor buildings using a one-dimensional optical fiber radiation sensor (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Nagoya University*

JAEA-Review 2022-033, 80 Pages, 2022/12

JAEA-Review-2022-033.pdf:4.08MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Measurement methods for the radioactive source distribution inside reactor buildings using a one-dimensional optical fiber radiation sensor" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. The present study aims to develop an optical fiber type radiation sensor that can measure the radiation distribution one-dimensionally along the fiber under a high radiation field for the decommissioning of 1F. Based on the conventional time-of-flight method, we found several promising sensor candidates for the radiation distribution measurement under high dose rate and many scattered gamma-rays.

Journal Articles

Characterization of bremsstrahlung and $$gamma$$-rays of fuel debris

Matsumura, Taichi; Okumura, Keisuke; Fujita, Manabu*; Sakamoto, Masahiro; Terashima, Kenichi; Riyana, E. S.

Radiation Physics and Chemistry, 199, p.110298_1 - 110298_8, 2022/10

 Times Cited Count:1 Percentile:31.61(Chemistry, Physical)

JAEA Reports

Measurement methods for the radioactive source distribution inside reactor buildings using a one-dimensional optical fiber radiation sensor (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Nagoya University*

JAEA-Review 2021-033, 55 Pages, 2021/12

JAEA-Review-2021-033.pdf:2.9MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Measurement methods for the radioactive source distribution inside reactor buildings using a one-dimensional optical fiber radiation sensor" conducted in FY2020. We are developing a one-dimensional optical fiber radiation sensor that can estimate the radioactive source distribution "along lines" instead of "at points". To improve the conventional time-of-flight optical fiber radiation sensor for the application under high dose rate environment, basic evaluation tests were conducted using various optical fibers with different diameters and materials.

JAEA Reports

Measurement methods for the radioactive source distribution inside reactor buildings using a one-dimensional optical fiber radiation sensor (Contract research); FY2019 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Nagoya University*

JAEA-Review 2020-063, 44 Pages, 2021/01

JAEA-Review-2020-063.pdf:2.55MB

JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project in FY2019. Among the adopted proposals in FY2019, this report summarizes the research results of the "Measurement methods for the radioactive source distribution inside reactor buildings using a one-dimensional optical fiber radiation sensor" conducted in FY2019.

Journal Articles

A New convention for the epithermal neutron spectrum for improving accuracy of resonance integrals

Harada, Hideo; Takayama, Naoki; Komeda, Masao

Journal of Physics Communications (Internet), 4(8), p.085004_1 - 085004_17, 2020/08

A new convention of epithermal neutron spectrum is formulated for improving accuracy of resonance integrals. The new type function is proposed as an approximating function of epithermal neutron spectrum based on calculations by the state-of-art Monte Carlo code MVP-3. Bias effects on determination of resonance integrals due to utilizing approximating functions of the traditional types and the new type are compared. The other bias effect is also investigated, which is caused by neglecting position dependence of a neutron spectrum inside an irradiation capsule. For demonstrating the bias effects due to these assumptions on neutron spectrum quantitatively in a practical case, the thermal neutron-capture cross section and resonance integral of $$^{135}$$Cs measured at a research reactor JRR-3 are re-evaluated. A superior property of the proposed new convention is discussed. The experimental method is proposed to determine the new shape factor $$beta$$ introduced in the convention by a combinational use of triple flux monitors ($$^{197}$$Au, $$^{59}$$Co and $$^{94}$$Zr), and its analytical methodology is formulated.

Journal Articles

Evaluation of energy spectrum around structural materials in radiation environments

Matsumura, Taichi; Nagaishi, Ryuji; Katakura, Junichi*; Suzuki, Masahide*

Radiation Physics and Chemistry, 166, p.108493_1 - 108493_9, 2020/01

 Times Cited Count:2 Percentile:12.16(Chemistry, Physical)

In this work, when radiation sources of $$^{137}$$Cs, $$^{90}$$Sr and $$^{90}$$Y were assumed to be put in the front of a plain SUS304 plate as a typical material submerged in water, energy spectra of secondary photons and electrons at the front and back sides of plate were simulated with changing the thickness of plate, and spacing between the source and plate by using a Monte Carlo calculation code of PHITS. In the case of $$^{137}$$Cs gamma-ray (monochromatic 662 keV), the energy spectra at the front side was smaller than those at the back side due to the existence of plate. Then the dependence of spectra on the plate thickness was observed more clearly at the back side than at the front side. It was clearly shown how the energy spectra of photons and electrons varied with the incident radiation type, the spacing, and the thickness.

Journal Articles

Calculation of gamma and neutron emission characteristics emitted from fuel debris of Fukushima Daiichi Nuclear Power Station

Riyana, E. S.; Okumura, Keisuke; Terashima, Kenichi

Journal of Nuclear Science and Technology, 56(9-10), p.922 - 931, 2019/09

 Times Cited Count:5 Percentile:48.99(Nuclear Science & Technology)

Journal Articles

Neutron spectrum change with thermal moderator temperature in a compact electron accelerator-driven neutron source and its effects on spectroscopic neutron transmission imaging

Ishikawa, Hirotaku*; Kai, Tetsuya; Sato, Hirotaka*; Kamiyama, Takashi*

Journal of Nuclear Science and Technology, 56(2), p.221 - 227, 2019/02

 Times Cited Count:3 Percentile:31.89(Nuclear Science & Technology)

Journal Articles

Continuous energy Monte Carlo criticality calculation of random media under power law spectrum

Ueki, Taro

Proceedings of International Conference on Mathematics and Computational Methods applied to Nuclear Science and Engineering (M&C 2019) (CD-ROM), p.151 - 160, 2019/00

A dynamical system under extreme physical disorder has the tendency of evolving toward the equilibrium state characterized by an inverse power law spectrum. In this paper, the author proposes a practically implementable modeling of random media under such a spectrum using a randomized form of the Weierstrass function. The proposed modeling is demonstrated by the continuous energy Monte Carlo particle transport with delta tracking for the criticality calculation of a randomized version of the Topsy spherical core in International Criticality Safety Benchmark Evaluation Project.

Journal Articles

Measurements of neutronic characteristics of rectangular and cylindrical coupled hydrogen moderators

Kai, Tetsuya; Kamiyama, Takashi*; Hiraga, Fujio*; Oi, Motoki; Hirota, Katsuya*; Kiyanagi, Yoshiaki*

Journal of Nuclear Science and Technology, 55(3), p.283 - 289, 2018/03

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

A Power spectrum approach to tally convergence in Monte Carlo criticality calculation

Ueki, Taro

Journal of Nuclear Science and Technology, 54(12), p.1310 - 1320, 2017/12

AA2017-0413.pdf:1.05MB

 Times Cited Count:6 Percentile:51.46(Nuclear Science & Technology)

In Monte Carlo criticality calculation, confidence interval estimation is based on the central limit theorem (CLT) for a series of tallies. A fundamental assertion resulting from CLT is the convergence in distribution (CID) of the interpolated standardized time series (ISTS) of tallies. In this work, the spectral analysis of ISTS has been conducted in order to assess the convergence of tallies in terms of CID. Numerical results indicate that the power spectrum of ISTS is equal to the theoretically predicted power spectrum of Brownian motion for effective neutron multiplication factor; on the other hand, the power spectrum of ISTS for local power fluctuates wildly while maintaining the spectral form of fractional Brownian motion. The latter result is the evidence of a case where a series of tallies is away from CID, while the spectral form supports normality assumption on the sample mean.

Journal Articles

Energy-resolved small-angle neutron scattering from steel

Oba, Yojiro*; Morooka, Satoshi; Oishi, Kazuki*; Suzuki, Junichi*; Takata, Shinichi; Sato, Nobuhiro*; Inoue, Rintaro*; Tsuchiyama, Toshihiro*; Gilbert, E. P.*; Sugiyama, Masaaki*

Journal of Applied Crystallography, 50(2), p.334 - 339, 2017/04

 Times Cited Count:3 Percentile:29.28(Chemistry, Multidisciplinary)

Journal Articles

Spectrum-dose conversion operator of NaI(Tl) and CsI(Tl) scintillation detectors for air dose rate measurement in contaminated environments

Tsuda, Shuichi; Saito, Kimiaki

Journal of Environmental Radioactivity, 166(Part 3), p.419 - 426, 2017/01

 Times Cited Count:27 Percentile:65.77(Environmental Sciences)

Air dose rate monitoring in the environment has been performed since the Fukushima Dai-ichi Nuclear Power Plant accident happened. In the measurement, NaI(Tl) and CsI(Tl) scintillation detectors are used, which are usually used in nuclear power plants and calibrated in a uniform irradiation condition in a radiation calibration field. In general, however, the detector responses are dependent on incident direction and in reality, the incident direction of the photons is not uniform in the environment. In this study, to evaluate the dependence of dose on the photon incident direction, the spectrum - dose conversion operator (G(E) function) for air kerma in a semi-infinite radiation field were obtained using the PHITS code for commonly used NaI(Tl) and CsI(Tl) scintillation detectors. The results indicate that the commonly used scintillation detectors overestimate the doses by a maximum of 40% for mono-energetic photons but under the real environment, one could obtain the dose in the semi-infinite radiation field within 20%.

JAEA Reports

Influence of fuel assembly loading pattern and fuel burnups upon leakage neutron flux spectra from light water reactor core (Joint research)

Kojima, Kensuke; Okumura, Keisuke; Kosako, Kazuaki*; Torii, Kazutaka*

JAEA-Research 2015-019, 90 Pages, 2016/01

JAEA-Research-2015-019.pdf:1.95MB

At the decommissioning of light water reactors (LWRs), it is important to evaluate an amount of radioactivity in the ex-core structures such as a reactor containment vessel, radiation shieldings, and so on. It is thought that the leakage neutron spectra in these radioactivation regions, which strongly affect the induced radioactivity, would be changed by different reactor core configurations such as fuel assembly loading pattern and fuel burnups. This study was intended to evaluate these effects. For the purpose, firstly, partial neutron currents on the core surfaces were calculated for some core configurations. Then, the leakage neutron flux spectra in major radioactivation regions were calculated based on the provided currents. Finally, influence of the core configurations upon the neutron flux spectra was evaluated. As a result, it has been found that the influence is small on the spectrum shapes of neutron fluxes. However, it is necessary to pay attention to the facts that intensities of the leakage neutron fluxes are changed by the configurations and that intensities and spectrum shapes of the leakage neutron fluxes are changed depending on the angular direction around the core.

Journal Articles

Desorption of cluster ions from frozen gases following high-density electronic excitation

Baba, Yuji; Sekiguchi, Tetsuhiro; Shimoyama, Iwao

Surface Science, 593(1-3), p.324 - 330, 2005/11

 Times Cited Count:6 Percentile:30.12(Chemistry, Physical)

no abstracts in English

JAEA Reports

Program POD-P; A Computer code to calculate cross sections for neutron-induced preequilibrium nuclear reactions

Kunieda, Satoshi; Ichihara, Akira

JAERI-Data/Code 2005-005, 33 Pages, 2005/09

JAERI-Data-Code-2005-005.pdf:1.5MB

The computer code, POD-P, was developed to calculate energy spectra and angular distributions of emitted particles for the neutron-induced preequiliblium nuclear reactions. The energy-differential cross sections are computed with the classical one-component exciton model for the nucleon and composite-particle emissions. Along with this, the semi-empirical exciton models are also used for the composite-particle emissions. The double-differential cross sections are derived from those model calculations plus the angular-distribution systematics. The computational method and explanation of input parameters are given with some output examples.

Journal Articles

Design of a single moderator-type neutron spectrometer with enhanced energy resolution in energy range from a few to 100 keV

Tanimura, Yoshihiko; Saegusa, Jun; Yoshizawa, Michio; Yoshida, Makoto

Nuclear Instruments and Methods in Physics Research A, 547(2-3), p.592 - 600, 2005/08

 Times Cited Count:8 Percentile:52.87(Instruments & Instrumentation)

The moderator structure of a neutron spectrometer was optimized with a Monte Carlo code of MCNP-4B. The spectrometer consists of a cylindrical moderator and a position-sensitive thermal neutron detector. It can obtain an energy spectrum from thermal neutron distribution along the cylindrical axis of the moderator. The structure of the moderator was improved by putting a low hydrogen density material in the front of a high hydrogen density one and inserting a neutron absorber which eliminated thermal neutrons diffusing in the moderator. These improvements make energy resolution of the spectrometer better especially for the low energy neutrons from a few tens to 100 keV. The designed spectrometer can be applied to the measurement of energy spectrum over a neutron energy range from a few keV to 20 MeV.

Journal Articles

Stabilization mechanism of ballooning modes by toroidal rotation shear in tokamaks

Furukawa, Masaru; Tokuda, Shinji

Nuclear Fusion, 45(5), p.377 - 383, 2005/05

 Times Cited Count:10 Percentile:34(Physics, Fluids & Plasmas)

A ballooning perturbation in a toroidally rotating tokamak is expanded by square-integrable eigenfunctions of an eigenvalue problem associated with ballooning modes in a static plasma. Especially a weight function is chosen such that the eigenvalue problem has only the discrete spectrum. The eigenvalues evolve in time owing to toroidal rotation shear, resulting in countably infinite number of crossings among them. The crossings cause energy transfer from an unstable mode to the infinite number of stable modes; such transfer works as the stabilization mechanism of the ballooning mode. A simple analytic formula is derived for estimating the toroidal rotation shear required to stabilize the ballooning mode.

189 (Records 1-20 displayed on this page)